'Single-photon emission enhancement' seen as step toward quantum technologies

January 13, 2015  


Nanodiamonds have been added to the surface of a new "hyperbolic metamaterial" to enhance the production of single photons, a step toward creating devices aimed at developing quantum computers and communications technologies. (Birck Nanotechnology Center image)

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WEST LAFAYETTE, Ind. - Researchers have demonstrated a new way to enhance the emission of single photons by using "hyperbolic metamaterials," a step toward creating devices in work aimed at developing quantum computers and communications technologies.

Optical metamaterials harness clouds of electrons called surface plasmons to manipulate and control light. Purdue University researchers had previously created "superlattices" from layers of the metal titanium nitride and the dielectric, or insulator, aluminum scandium nitride. Unlike some of the plasmonic components under development, which rely on the use of noble metals such as gold and silver, the new metamaterial is compatible with the complementary metal–oxide–semiconductor manufacturing process used to construct integrated circuits.

The metamaterial is said to be hyperbolic, meaning it possesses unique properties leading to the increased output of light. In new findings the researchers have demonstrated how attaching nanodiamonds containing "nitrogen-vacancy centers" to the new metamaterial further enhances the production of single photons, workhorses of quantum information processing, which could bring superior computers, cryptography and communications technologies.

"These results indicate that the brightness of the nanodiamond-based single-photon emitter could be substantially enhanced by placing such an emitter on the surface of the hyperbolic metamaterial," said Alexander Kildishev, associate professor of electrical and computer engineering at Purdue. "The single-photon emitters could be used to build highly efficient room temperature CMOS-compatible single-photon sources."

Research findings are detailed in a cover paper appearing in the Jan. 15 issue of Laser & Photonics Reviews. The work was a collaboration of researchers from Purdue, the Russian Quantum Center, Moscow Institute of Physics and Technology, Lebedev Physical Institute, and Photonic Nano-Meta Technologies Inc.

A nitrogen-vacancy center is an atomic-scale defect formed in the diamond lattice by substituting a nitrogen atom for a carbon atom and creating a neighboring void in the lattice. Placing a nanodiamond containing an NV center on the surface of hyperbolic metamaterials not only enhances the emission of photons, but also changes the pattern of light emitted, a trait that could be important for the development of quantum devices, said graduate student Mikhail Y. Shalaginov, the paper's lead author. He and Kildishev are working with a team of researchers led by Vladimir M. Shalaev, scientific director of nanophotonics at Purdue's Birck Nanotechnology Center and a distinguished professor of electrical and computer engineering, and Alexandra Boltasseva, an associate professor of electrical and computer engineering. Professors Shalaev, Kildishev and Boltasseva are a part of a Purdue "preeminent team" working on quantum photonics.

Because the studied system represents a stable source of single photons that functions at room temperature, it is potentially practical for commercial applications. When exposed to a laser light, the system rises from its "ground state" to an excited state, which causes it to spontaneously emit a photon.

"We are interested in causing it to emit faster so that we can increase the rate of these photons coming out," Kildishev said.

Findings show the system is capable of producing single photons faster, in larger quantities, and more directionally.

Metamaterials have engineered surfaces that contain features, patterns or elements, such as tiny antennas or alternating layers of nitrides that enable unprecedented control of light. Constructed of artificial atoms and molecules, the optical metamaterials owe their unusual potential to precision engineering on the scale of nanometers.

Quantum computers would take advantage of phenomena described by quantum theory called "superposition" and "entanglement." Instead of only the states of one and zero that exist in conventional computers, there are many possible "superposition quantum states." Computers based on quantum physics would have quantum bits, or "qubits," increasing the computer's capacity to process, store, and transmit information. The nitrogen vacancy also makes it possible to potentially record information based on the nuclear or electron "spin" state of the center, which is promising for quantum computing. The spin can be either "up" or "down" - forming the quantum superposition of the up and down states - representing a new technology for processing information.

Future research may include work to improve the system with devices that combine the hyperbolic metamaterial with nanoantennas and optical waveguides to increase its efficiency and make it more compact. The ongoing work also may strive to improve the "spin properties" of the system with nitrogen-vacancies and to study the optical contrast between the up and down states.

The research paper was authored by Shalaginov; graduate students Vadim V. Vorobyov and Jing Liu; Marcello Ferrera, a visiting researcher from Heriot-Watt University in the UK; Alexey V. Akimov, a researcher from the Moscow Institute of Physics, Russian Quantum Center and Lebedev Physical Institute; Purdue research scientist Alexei Lagutchev; Andrey N. Smolyaninov, a researcher from Photonic Nano-Meta Technologies, Russia; Vasily V. Klimov, from Lebedev Physical Institute and Photonic Nano-Meta Technologies; Joseph Irudayaraj, a Purdue professor of biological engineering and deputy director of the Bindley Bioscience Center; Kildishev, Boltasseva and Shalaev.

Writer: Emil Venere, 765-494-4709, venere@purdue.edu

Sources: Alexander Kildishev, 765-496-3196, kildishev@purdue.edu

Vladimir Shalaev, 765-494-9855, shalaev@ecn.purdue.edu

Alexandra Boltasseva, 765-494-0301, aeb@purdue.edu

Mikhail Y. Shalaginov, shalaginov@purdue.edu 


Enhancement of single–photon emission from nitrogen–vacancy centers with TiN/(Al,Sc)N hyperbolic metamaterial

Mikhail Y. Shalaginov 1,2,∗∗, Vadim V. Vorobyov 3,4,∗∗, Jing Liu5, Marcello Ferrera 1,2,7, Alexey V. Akimov 4,6,8, Alexei Lagutchev 2, Andrey N. Smolyaninov 3, Vasily V. Klimov 3,8, Joseph Irudayaraj5, Alexander V. Kildishev 1,2, Alexandra Boltasseva 1,2, and Vladimir M. Shalaev, 1,2, ,

1 School of Electrical and Computer Engineering, Purdue University

2 Birck Nanotechnology Center, Purdue University

3 Photonic Nano-Meta Technologies, ul. Lugovaya 4, Skolkovo Innovation Center, Moscow

4 Moscow Institute of Physics and Technology, Institutskiy per. 9, Dolgoprudny, Moscow Region

5 Agricultural and Biological Engineering, Purdue University

6 Russian Quantum Center

7 School of Engineering and Physical Sciences, Heriot-Watt University, Edinburgh, Scotland

8 Lebedev Physical Institute

**These authors contributed equally to this work.

∗Corresponding author: E-mail: shalaev@purdue.edu 

The broadband enhancement of single-photon emission from nitrogen-vacancy centers in nanodiamonds coupled to a planar multilayer metamaterial with hyperbolic dispersion is studied experimentally. The metamaterial is fabricated as an epitaxial metal/dielectric superlattice consisting of CMOS-compatible ceramics: titanium nitride (TiN) and aluminum scandium nitride (AlxSc1-xN). It is demonstrated that employing the metamaterial results in significant enhancement of collected single-photon emission and reduction of the excited-state lifetime. Our results could have an impact on future CMOS-compatible integrated quantu quantum sources.

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